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Abstract Bismuth ferrite (BiFeO3) is a multiferroic material that exhibits both ferroelectricity and canted antiferromagnetism at room temperature, making it a unique candidate in the development of electric-field controllable magnetic devices. The magnetic moments in BiFeO3are arranged into a spin cycloid, resulting in unique magnetic properties which are tied to the ferroelectric order. Previous understanding of this coupling has relied on average, mesoscale measurements. Using nitrogen vacancy-based diamond magnetometry, we observe the magnetic spin cycloid structure of BiFeO3in real space. This structure is magnetoelectrically coupled through symmetry to the ferroelectric polarization and this relationship is maintained through electric field switching. Through a combination of in-plane and out-of-plane electrical switching, coupled with ab initio studies, we have discovered that the epitaxy from the substrate imposes a magnetoelastic anisotropy on the spin cycloid, which establishes preferred cycloid propagation directions. The energy landscape of the cycloid is shaped by both the ferroelectric degree of freedom and strain-induced anisotropy, restricting the spin spiral propagation vector to changes to specific switching events.more » « lessFree, publicly-accessible full text available December 1, 2025
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Abstract Stabilization of topological spin textures in layered magnets has the potential to drive the development of advanced low-dimensional spintronics devices. However, achieving reliable and flexible manipulation of the topological spin textures beyond skyrmion in a two-dimensional magnet system remains challenging. Here, we demonstrate the introduction of magnetic iron atoms between the van der Waals gap of a layered magnet, Fe3GaTe2, to modify local anisotropic magnetic interactions. Consequently, we present direct observations of the order-disorder skyrmion lattices transition. In addition, non-trivial topological solitons, such as skyrmioniums and skyrmion bags, are realized at room temperature. Our work highlights the influence of random spin control of non-trivial topological spin textures.more » « lessFree, publicly-accessible full text available December 1, 2025
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null (Ed.)The implementation of full-duplex (FD) theoretically doubles the spectral efficiency of cellular communications. We propose a multiuser FD cellular network relying on an intelligent reflecting surface (IRS). The IRS is deployed to cover a dead zone while suppressing user-side self-interference (SI) and co-channel interference (CI) by carefully tuning the phase shifts of its massive low-cost passive reflection elements. To ensure network fairness, we aim to maximize the weighted minimum rate (WMR) of all users by jointly optimizing the precoding matrix of the base station (BS) and the reflection coefficients of the IRS. Specifically, we propose a low-complexity minorization-maximization (MM) algorithm for solving the subproblems of designing the precoding matrix and the reflection coefficients, respectively. Simulation results confirm the convergence and efficiency of our proposed algorithm, and validate the advantages of introducing IRS to realize FD cellular communications.more » « less
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Abstract Highly responsive, voltage‐tunable dielectrics are essential for microwave‐telecommunication electronics. Ferroelectric/relaxor materials have been leading candidates for such functionality and have exhibited agile dielectric responses. Here, it is demonstrated that relaxor materials developed from antiferroelectrics can achieve both ultrahigh dielectric response and tunability. The system, based on alloying the archetypal antiferroelectric PbZrO3with the dielectric BaZrO3, exhibits a more complex phase evolution than that in traditional relaxors and is characterized by an unconventional multi‐phase competition between antiferroelectric, ferroelectric, and paraelectric order. This interplay of phases can greatly enhance the local heterogeneities and results in relaxor characteristics while preserving considerable polarizability. Upon studying Pb1‐xBaxZrO3forx= 0‐0.45, Pb0.65Ba0.35ZrO3is found to provide for exceptional dielectric tunability under low bias fields (≈81% at 200 kV cm−1and ≈91% at 500 kV cm−1) at 10 kHz, outcompeting most traditional relaxor ferroelectric films. This high tunability is sustained in the radio‐frequency range, resulting in a high commutation quality factor (>2000 at 1 GHz). This work highlights the phase evolution from antiferroelectrics (with lower, “positive” dielectric tunability) to relaxors (with higher, “negative” tunability), underscoring a promising approach to develop relaxors with enhanced functional capabilities and new possibilities.more » « less
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